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Chapter 1 Project Overview 1£®1 Introduction 1£®1£®1 Overall Arrangement 1£®1£®2 Overview of Program Implementation 1£®1£®3 Interdisciplinary Efforts 1£®2 Research Circumstances 1£®2£®1 Overall Scientific Objectives 1£®2£®2 Key Scientific Issues 1£®3 Significant Progress Chapter 2 Research in China and Abroad 2£®1 Research Status and Development Trend 2£®1£®1 Research Status and Development Trend of Optoelectronic Functional Crystals 2£®1£®2 Research Status and Development Trend of Molecular Ferroelectrics 2£®1£®3 Research Status and Development Trend of Molecular Magnetics 2£®1£®4 Research Status and Development Trend of Superconducting Materials 2£®1£®5 Research Status and Development Trend of Thermoelectric Materials 2£®2 Development Trends of Functional Crystalline Materials 2£®2£®1 Developments in Laser Crystals and Nonlinear Optical Crystals 2£®2£®2 Development Trend of Molecular Ferroelectrics 2£®2£®3 Development Trend of Molecular Magnets 2£®2£®4 Development Trend of Metal-Organic Framework Materials 2£®2£®5 Development Trend of Superconducting Materials 2£®2£®6 Trends in Thermoelectric Materials Chapter 3 Major Research Achievements 3£®1 Structural Designing and Modulation of Magnetic Functional Molecular Crystalline Materials 3£®1£®1 Ground-State Spin and Uniaxial Magnetic Anisotropy Modulation of Single-Molecule Magnets 3£®1£®2 Metal-Organic Single-Ion Magnets 3£®1£®3 Assembly Based on High-Performance Single-Ion Magnet Substrates 3£®1£®4 Nuclear Spin Strategy for Suppressing Magnetic Quantum Tunneling Effect 3£®2 Design£¬ Synthesis£¬ and Performance of High-Performance Molecular Ferroelectrics 3£®2£®1 Molecular Ferroelectrics with High Curie Temperature£¬ Large Saturation Polarization 3£®2£®2 Molecular Ferroelectrics with Large Piezoelectric Coefficients 3£®2£®3 Homochiral Molecular Ferroelectrics 3£®2£®4 Molecular Ferroelectrics with Semiconductor Properties 3£®2£®5 New Strategies for Precise Design of Molecular Ferroelectrics 3£®2£®6 Photoferroelectric Semiconductor Crystalline Materials for Next-Generation Photoelectric Detection Technology 3£®2£®7 Discovery of Molecule-Based Ferroelectric Crystalline Materials with Fast Polarization Reversals 3£®2£®8 Discovery of Incommensurate Structure Modulated Molecular Ferroelectric Crystals 3£®3 Laser Crystals and Nonlinear Optical Crystals 3£®3£®1 Research on the Structure-Property Relationships of Nonlinear Optical Crystals 3£®3£®2 New Deep-Ultraviolet Nonlinear Optical Crystals 3£®3£®3 Infrared Nonlinear Optical Crystal 3£®3£®4 Laser Crystals and Transparent Ceramics 3£®4 New Electron-Doped Iron-Selenium-Based Superconductors 3£®4£®1 First Discovery of Electron-Doped Iron-Selenium-Based Superconductors 3£®4£®2 First Discovery of Molecular Intercalation Series of Iron-Selenium- Based High-Temperature Superconductors 3£®4£®3 True Composition and Structure of Superconducting Phases in the K-Fe-Se System 3£®4£®4 First Anderson Localization in the Single-Crystal Electron System 3£®4£®5 Regulation of Superconductivity in \"l-hin-Layered Iron-Selenium £¨FeSe£© Single-Crystals 3£®5 Other Novel Crystalline Materials 3£®5£®1 Metal-Organic Framework Isoporous Materials 3£®5£®2 2D Crystalline Materials Chapter 4 Outlook 4£®1 Strategic Needs 4£®2 Conceptions and Suggestions References Index